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Some research on a theory of the structural composition of an algorithm has recently been reported. The theory embodies models of operator and operand distributions that have been proposed by Bayer, Zipf, and Zweben. This paper reports a study in which the three models of operator distributions are compared with the measured distributions found in 34 PL/I programs. Two of three models, one by Zipf and one by Zweben, are shown to correlate highly with the measured distributions. Two variations of the Zipf model are then formulated and tested with good results. Also, the relationship between the method of counting operators and the models is investigated.