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This paper shows how predicate equation systems (PESs) may be used to solve model-checking problems for systems, such as those involving real-time or value passing, that manipulate data. PESs are first defined and the encoding of model-checking problems described; then generic global and local approaches for solving PESs are given. Real-time model checking is then considered in detail, and a new, efficient on-the-fly technique for real-time model checking based on proof search in PESs is developed and experimentally shown to significantly outperform existing approaches when system specifications or formula specifications contain errors and to be competitive when both are correct.